unfasten v 1: cause to become undone; "unfasten your belt" [ant: {fasten}, {fix}, {secure}] 2: become undone or untied; "The shoelaces unfastened" [ant: {fasten}]
Unfasten \Un*fas"ten\, v. t. [1st pref. un- + fasten.] To loose; to unfix; to unbind; to untie. [1913 Webster]
31 Moby Thesaurus words for "unfasten": cast off, detach, disengage, doff, free, liberate, loose, loosen, release, remove, take off, unbar, unbind, unbolt, unbuckle, unbutton, unchain, unclasp, undo, unfetter, unglue, unlace, unlatch, unleash, unlock, unloose, unloosen, unstick, unstrap, untie, weigh anchor